Quantum Oscillations
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In condensed matter physics, quantum oscillations describes a series of related
experimental An experiment is a procedure carried out to support or refute a hypothesis, or determine the efficacy or likelihood of something previously untried. Experiments provide insight into cause-and-effect by demonstrating what outcome occurs when a ...
techniques used to map the
Fermi surface In condensed matter physics, the Fermi surface is the surface in reciprocal space which separates occupied from unoccupied electron states at zero temperature. The shape of the Fermi surface is derived from the periodicity and symmetry of the crys ...
of a
metal A metal (from Greek μέταλλον ''métallon'', "mine, quarry, metal") is a material that, when freshly prepared, polished, or fractured, shows a lustrous appearance, and conducts electricity and heat relatively well. Metals are typicall ...
in the presence of a strong magnetic field. These techniques are based on the principle of
Landau quantization In quantum mechanics, Landau quantization refers to the quantization of the cyclotron orbits of charged particles in a uniform magnetic field. As a result, the charged particles can only occupy orbits with discrete, equidistant energy values, call ...
of
Fermions In particle physics, a fermion is a particle that follows Fermi–Dirac statistics. Generally, it has a half-odd-integer spin: spin , spin , etc. In addition, these particles obey the Pauli exclusion principle. Fermions include all quarks and ...
moving in a magnetic field. For a gas of free fermions in a strong magnetic field, the energy levels are quantized into bands, called the ''Landau levels'', whose separation is proportional to the strength of the magnetic field. In a quantum oscillation experiment, the external magnetic field is varied, which causes the Landau levels to pass over the Fermi surface, which in turn results in oscillations of the electronic
density of states In solid state physics and condensed matter physics, the density of states (DOS) of a system describes the number of modes per unit frequency range. The density of states is defined as D(E) = N(E)/V , where N(E)\delta E is the number of states i ...
at the Fermi level; this produces oscillations in the many material properties which depend on this, including resistance (the
Shubnikov–de Haas effect An oscillation in the conductivity of a material that occurs at low temperatures in the presence of very intense magnetic fields, the Shubnikov–de Haas effect (SdH) is a macroscopic manifestation of the inherent quantum mechanical nature of matter ...
), Hall resistance, and magnetic susceptibility (the de Haas–van Alphen effect). Observation of quantum oscillations in a material is considered a signature of
Fermi liquid Fermi liquid theory (also known as Landau's Fermi-liquid theory) is a theoretical model of interacting fermions that describes the normal state of most metals at sufficiently low temperatures. The interactions among the particles of the many-body ...
behaviour. Quantum oscillations have been used to study high temperature superconducting materials such as cuprates and pnictides. Studies using these experiments have shown that the ground state of underdoped cuprates behave similar to a
Fermi liquid Fermi liquid theory (also known as Landau's Fermi-liquid theory) is a theoretical model of interacting fermions that describes the normal state of most metals at sufficiently low temperatures. The interactions among the particles of the many-body ...
, and display characteristics such as Landau
quasiparticle In physics, quasiparticles and collective excitations are closely related emergent phenomena arising when a microscopically complicated system such as a solid behaves as if it contained different weakly interacting particles in vacuum. For exa ...
s. In 2021 this technique has been used to observe a predicted state called "electron–phonon fluid", a similar particle-quasiparticle state already known is the exciton–polariton fluid.


Experiment

When a magnetic field is applied to a system of free charged
fermions In particle physics, a fermion is a particle that follows Fermi–Dirac statistics. Generally, it has a half-odd-integer spin: spin , spin , etc. In addition, these particles obey the Pauli exclusion principle. Fermions include all quarks and ...
, their energy states are quantized into the so-called Landau levels, given by \varepsilon_l=\frac\left(\ell +\frac\right) for integer-valued \ell, where B is the external magnetic field and e,m^* are the fermion charge and effective mass respectively. When the external magnetic field B is increased in an isolated system, the Landau levels expand, and eventually "fall off" the Fermi surface. This leads to oscillations in the observed energy of the highest occupied level, and hence in many physical properties (including Hall conductivity, resistivity, and susceptibility). The periodicity of these oscillations can be measured, and in turn can be used to determine the cross-sectional area of the Fermi surface. If the axis of the magnetic field is varied at constant magnitude, similar oscillations are observed. The oscillations occur whenever the Landau orbits touch the Fermi surface. In this way, the complete geometry of the Fermi sphere can be mapped.


Underdoped cuprates

Studies of underdoped cuprate compounds such as YBa2Cu3O6+''x'' through probes such as
ARPES Angle-resolved photoemission spectroscopy (ARPES) is an experimental technique used in condensed matter physics to probe the allowed energies and momenta of the electrons in a material, usually a crystalline solid. It is based on the photoelec ...
have indicated that these phases show characteristics of non-Fermi liquids, and in particular, the absence of well-defined Landau
quasiparticle In physics, quasiparticles and collective excitations are closely related emergent phenomena arising when a microscopically complicated system such as a solid behaves as if it contained different weakly interacting particles in vacuum. For exa ...
s.{{cite journal, last1=Damascelli, first1=Andrea, last2=Hussain, first2=Zahid, author3=Zhi-Xun Shen, title=Angle-resolved photoemission studies of the cuprate superconductors, journal=Reviews of Modern Physics, year=2003, volume=75, issue=2, pages=473, doi=10.1103/RevModPhys.75.473, arxiv = cond-mat/0208504 , bibcode = 2003RvMP...75..473D , s2cid=118433150 However, quantum oscillations have been observed in these materials at low temperatures, if their superconductivity is suppressed by a sufficiently high magnetic field, which is evidence for the presence of well-defined quasiparticles with fermionic statistics. These experimental results thus disagree with those from ARPES and other probes.


See also

* de Haas–van Alphen effect *
Shubnikov–de Haas effect An oscillation in the conductivity of a material that occurs at low temperatures in the presence of very intense magnetic fields, the Shubnikov–de Haas effect (SdH) is a macroscopic manifestation of the inherent quantum mechanical nature of matter ...
* Landau levels


References

Condensed matter physics Experimental physics Magnetism